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We report charge transfer and built-in electric fields across the epitaxial SrNbxTi1−xO3−δ=Sið001Þ interface. Electrical transport measurements indicate the formation of a hole gas in the Si and the presence of built-in fields. Hard x-ray photoelectron measurements reveal pronounced asymmetries in core-level spectra that arise from these built-in fields. Theoretical analysis of core-level spectra enables built-in fields and the resulting band bending to be spatially mapped across the heterojunction. The demonstration of tunable charge transfer, built-in fields, and the spatial mapping of the latter, lays the groundwork for the development of electrically coupled, functional heterojunctions.more » « less
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Lim, Z. H. ; Quackenbush, N. F. ; Penn, A. N. ; Chrysler, M. ; Bowden, M. ; Zhu, Z. ; Ablett, J. M. ; Lee, T. -L. ; LeBeau, J. M. ; Woicik, J. C. ; et al ( , Physical Review Letters)
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Huang, C-Y ; Zhou, J. ; Tra, V. T. ; White, R. ; Trappen, R. ; N’Diaye, A. T. ; Spencer, M. ; Frye, C. ; Cabrera, G. B. ; Nguyen, V. ; et al ( , Journal of Physics: Condensed Matter)
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Lim, Z. H. ; Ahmadi-Majlan, K. ; Grimley, E. D. ; Du, Y. ; Bowden, M. ; Moghadam, R. ; LeBeau, J. M. ; Chambers, S. A. ; Ngai, J. H. ( , Journal of Applied Physics)